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Is it possible to block outgoing calls from my Plusnet landline to a specific mobile number or alternatively, to mobile numbers in general?
Go to the fix.
Plusnet offer call barring for various types of call.
Unfortunately the only way to bar mobiles is to opt for 'International calls and calls to mobiles'.
See 'How do I use call features' here - https://www.plus.net/help/phone/call-features/
Once logged into the Member Centre, you call add call features here - https://www.plus.net/member-centre/phone/call-features
There is an ongoing problem with that page, inasmuch as you can't scroll down to the bottom of the page to see 'Call barring'.
Depending on your screen size and resolution, you might manage it by zooming out with your browser.